High time resolution spectroscopy studies of the explosive decomposition of silver azide / B. P. Aduev [et al.]

Уровень набора: Russian Physics Journal = 1965-Альтернативный автор-лицо: Aduev, B. P.;Aluker, E. D.;Belokurov, G. M.;Zakharov, Yu. A., Russian chemist, Doctor of Chemical Sciences, Professor of Tomsk Polytechnic University, 1938 -, Yuriy Aleksandrovich;Krechetov, A. G.Язык: английский.Резюме или реферат: We have analyzed the existing assumptions about the mechanism of the explosive decomposition of the heavy metal azides. We present here a study of the kinetics of the explosive decomposition of silver azide, initiated by a laser pulse. New effects are identified and studied, including a pre-explosion conductivity and luminescence. On the basis of our results, we conclude that the reaction proceeds by a chain reaction mechanism. In terms of band theory, we propose a model of the primary chain step of the reaction as the creation of a quasilocalized state deep in the valence band with two holes localized at a defect (N30), with impact ionization occurring as they “float up”..Примечания о наличии в документе библиографии/указателя: [References: p. 1145 (23 tit.)].Аудитория: .Тематика: электронный ресурс | труды учёных ТПУ | спектроскопия | азид серебра Ресурсы он-лайн:Щелкните здесь для доступа в онлайн
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Title screen

[References: p. 1145 (23 tit.)]

We have analyzed the existing assumptions about the mechanism of the explosive decomposition of the heavy metal azides. We present here a study of the kinetics of the explosive decomposition of silver azide, initiated by a laser pulse. New effects are identified and studied, including a pre-explosion conductivity and luminescence. On the basis of our results, we conclude that the reaction proceeds by a chain reaction mechanism. In terms of band theory, we propose a model of the primary chain step of the reaction as the creation of a quasilocalized state deep in the valence band with two holes localized at a defect (N30), with impact ionization occurring as they “float up”.

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