Oxidative addition of verdazyl halogenides to Pd(PPh3)4 / P. V. Petunin, D. E. Votkina, M. E. Trusova [et al.]

Уровень набора: New Journal of ChemistryАльтернативный автор-лицо: Petunin, P. V., chemist, Engineer of Tomsk Polytechnic University, 1982-, Pavel Vasilievich;Votkina, D. E., chemical engineer, Engineer of the Tomsk Polytechnic University, 1995-, Darjya Evgenjevna;Trusova, M. E., organic chemist, Associate professor of Tomsk Polytechnic University, Candidate of chemical sciences, 1982-, Marina Evgenievna;Rybalova, T. V., Tatjyana Valerjevna;Amosov, E. V., Evgeny Valerjevich;Uvarov, M. N., Mikhail Nikolaevich;Postnikov, P. S., organic chemist, Associate Professor of Tomsk Polytechnic University, Candidate of chemical sciences, 1984-, Pavel Sergeevich;Kazantsev, M. S., Maksim Sergeevich;Mostovich, E. A., Evgeny AlekseevichКоллективный автор (вторичный): Национальный исследовательский Томский политехнический университет, Исследовательская школа химических и биомедицинских технологий (ИШХБМТ), (2017- )Язык: английский.Резюме или реферат: Direct oxidative addition of verdazyl halogenides to Pd(0) was studied and the role of this step in the Pd-catalyzed cross-coupling reactions was evaluated. A number of bis(triphenylphosphine)[verdazyl]palladium(II) iodide species were synthesized in yields of 89 to 92% and were shown to be persistent under ambient conditions. High synthetic potential of Pd-verdazyls was demonstrated by their efficiency and reactivity in the Sonogashira coupling reaction. These derivatives significantly expand the modern synthetic tools for development of spin-labeled materials and polyradical systems with desired functionalities..Аудитория: .Тематика: электронный ресурс | труды учёных ТПУ | окислительное присоединение Ресурсы он-лайн:Щелкните здесь для доступа в онлайн
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Direct oxidative addition of verdazyl halogenides to Pd(0) was studied and the role of this step in the Pd-catalyzed cross-coupling reactions was evaluated. A number of bis(triphenylphosphine)[verdazyl]palladium(II) iodide species were synthesized in yields of 89 to 92% and were shown to be persistent under ambient conditions. High synthetic potential of Pd-verdazyls was demonstrated by their efficiency and reactivity in the Sonogashira coupling reaction. These derivatives significantly expand the modern synthetic tools for development of spin-labeled materials and polyradical systems with desired functionalities.

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