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100 _a20161020a2016 k y0engy50 ba
101 0 _aeng
_deng
102 _aUS
135 _adrcn ---uucaa
181 0 _ai
182 0 _ab
200 1 _aMatrix association effects on hydrodynamic sorting and degradation of terrestrial organic matter during cross-shelf transport in the Laptev and East Siberian shelf seas
_fT. Tesi [et al.]
203 _aText
_celectronic
300 _aTitle screen
330 _aThis study seeks an improved understanding of how matrix association affects the redistribution and degradation of terrigenous organic carbon (TerrOC) during cross-shelf transport in the Siberian margin. Sediments were collected at increasing distance from two river outlets (Lena and Kolyma Rivers) and one coastal region affected by erosion. Samples were fractionated according to density, size, and settling velocity. The chemical composition in each fraction was characterized using elemental analyses and terrigenous biomarkers. In addition, a dual-carbon-isotope mixing model (d13C and ?14C) was used to quantify the relative TerrOC contributions from active layer (Topsoil) and Pleistocene Ice Complex Deposits (ICD). Results indicate that physical properties of particles exert first-order control on the redistribution of different TerrOC pools. Because of its coarse nature, plant debris is hydraulically retained in the coastal region. With increasing distance from the coast, the OC is mainly associated with fine/ultrafine mineral particles. Furthermore, biomarkers indicate that the selective transport of fine-grained sediment results in mobilizing high-molecular weight (HMW) lipid-rich, diagenetically altered TerrOC while lignin-rich, less degraded TerrOC is retained near the coast. The loading (µg/m2) of lignin and HMW wax lipids on the fine/ultrafine fraction drastically decreases with increasing distance from the coast (98% and 90%, respectively), which indicates extensive degradation during cross-shelf transport. Topsoil-C degrades more readily (90?±?3.5%) compared to the ICD-C (60?±?11%) during transport. Altogether, our results indicate that TerrOC is highly reactive and its accelerated remobilization from thawing permafrost followed by cross-shelf transport will likely represent a positive feedback to climate warming.
333 _aРежим доступа: по договору с организацией-держателем ресурса
461 _tJournal of Geophysical Research: Biogeosciences
463 _tVol. 121, iss. 3
_v[P. 731-752]
_d2016
610 1 _aэлектронный ресурс
610 1 _aтруды учёных ТПУ
701 1 _aTesi
_bT.
_gTommaso
701 1 _aSemiletov
_bI. P.
_cgeographer
_cProfessor of Tomsk Polytechnic University, doctor of geographical Sciences
_f1955-
_gIgor Petrovich
_2stltpush
_3(RuTPU)RU\TPU\pers\34220
701 1 _aDudarev
_bO. V.
_cgeologist
_cresearcher of Tomsk Polytechnic University, candidate of geological and mineralogical Sciences
_f1955-
_gOleg Viktorovich
_2stltpush
_3(RuTPU)RU\TPU\pers\35379
701 1 _aAndersson
_bA.
_gAugust
701 1 _aGustafsson
_bO.
_gOrjan
712 0 2 _aНациональный исследовательский Томский политехнический университет (ТПУ)
_bИнститут природных ресурсов (ИПР)
_bКафедра геологии и разведки полезных ископаемых (ГРПИ)
_bМеждународная научно-образовательная лаборатория изучения углерода арктических морей (МНОЛ ИУАМ)
_h7398
_2stltpush
_3(RuTPU)RU\TPU\col\20711
712 0 2 _aНациональный исследовательский Томский политехнический университет (ТПУ)
_bИнститут природных ресурсов (ИПР)
_bКафедра геологии и разведки полезных ископаемых (ГРПИ)
_bМеждународная научно-образовательная лаборатория изучения углерода арктических морей (МНОЛ ИУАМ)
_h7398
_2stltpush
_3(RuTPU)RU\TPU\col\20711
801 2 _aRU
_b63413507
_c20170209
_gRCR
856 4 _uhttp://dx.doi.org/10.1002/2015JG003067
942 _cCF