| 000 | 03568nlm1a2200577 4500 | ||
|---|---|---|---|
| 001 | 665262 | ||
| 005 | 20231030041957.0 | ||
| 035 | _a(RuTPU)RU\TPU\network\36461 | ||
| 035 | _aRU\TPU\network\36048 | ||
| 090 | _a665262 | ||
| 100 | _a20210907a2021 k y0engy50 ba | ||
| 101 | 0 | _aeng | |
| 102 | _aGB | ||
| 135 | _adrcn ---uucaa | ||
| 181 | 0 | _ai | |
| 182 | 0 | _ab | |
| 200 | 1 |
_aExploring the 3D structure and defects of a self-assembled gold mesocrystal by coherent X-ray diffraction imaging _fJ. Carnis, F. Kirner, D. Lapkin [et al.] |
|
| 203 |
_aText _celectronic |
||
| 300 | _aTitle screen | ||
| 320 | _a[References: 58 tit.] | ||
| 330 | _aMesocrystals are nanostructured materials consisting of individual nanocrystals having a preferred crystallographic orientation. On mesoscopic length scales, the properties of mesocrystals are strongly affected by structural heterogeneity. Here, we report the detailed structural characterization of a faceted mesocrystal grain self-assembled from 60 nm sized gold nanocubes. Using coherent X-ray diffraction imaging, we determined the structure of the mesocrystal with the resolution sufficient to resolve each gold nanoparticle. The reconstructed electron density of the gold mesocrystal reveals its intrinsic structural heterogeneity, including local deviations of lattice parameters, and the presence of internal defects. The strain distribution shows that the average superlattice obtained by angular X-ray cross-correlation analysis and the real, “multidomain” structure of a mesocrystal are very close to each other, with a deviation less than 10%. These results will provide an important impact to understanding the fundamental principles of structuring and self-assembly including ensuing properties of mesocrystals. | ||
| 461 | _tNanoscale | ||
| 463 |
_tVol. 13, iss. 23 _v[P. 9449-9892] _d2021 |
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| 610 | 1 | _aэлектронный ресурс | |
| 610 | 1 | _aтруды учёных ТПУ | |
| 610 | 1 | _aтрехмерные структуры | |
| 610 | 1 | _aдефекты | |
| 610 | 1 | _aзолото | |
| 610 | 1 | _aрентгеновская дифракция | |
| 610 | 1 | _aнаноструктурированные материалы | |
| 610 | 1 | _aнанокристаллы | |
| 610 | 1 | _aмезокристаллы | |
| 701 | 1 |
_aCarnis _bJ. _gJerome |
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| 701 | 1 |
_aKirner _bF. _gFelizitas |
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| 701 | 1 |
_aLapkin _bD. _gDmitry |
|
| 701 | 1 |
_aSturm _bS. _gSebastian |
|
| 701 | 0 | _aKim Young Yong | |
| 701 | 1 |
_aBaburin _bI. A. _gIgor |
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| 701 | 1 |
_aKhubbutdinov _bR. M. _gRuslan |
|
| 701 | 1 |
_aIgnatenko _bA. |
|
| 701 | 1 |
_aYashina _bE. G. _gEkaterina Gennadjevna |
|
| 701 | 1 |
_aMistonov _bA. A. _gAleksandr Andreevich |
|
| 701 | 1 |
_aSteegemans _bT. _gTristan |
|
| 701 | 1 |
_aWieck _bT. _gThomas |
|
| 701 | 1 |
_aGemming _bT. _gThomas |
|
| 701 | 1 |
_aLubk _bA. _gAxel |
|
| 701 | 1 |
_aLazarev _bS. V. _cphysicist _cengineer at Tomsk Polytechnic University _f1984- _gSergey Vladimirovich _2stltpush _3(RuTPU)RU\TPU\pers\35210 |
|
| 712 | 0 | 2 |
_aНациональный исследовательский Томский политехнический университет _bИнженерная школа неразрушающего контроля и безопасности _bЦентр промышленной томографии _bМеждународная научно-образовательная лаборатория неразрушающего контроля _h6776 _2stltpush _3(RuTPU)RU\TPU\col\19961 |
| 801 | 2 |
_aRU _b63413507 _c20210907 _gRCR |
|
| 856 | 4 | _uhttps://doi.org/10.1039/D1NR01806J | |
| 942 | _cCF | ||