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101 0 _aeng
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181 0 _ai
182 0 _ab
200 1 _aElectron Correlations in Sequential Two-Photon Double Ionization of an Ar Atom
_fB. M. Lagutin, I. D. Petrov, V. L. Sukhorukov [et al.]
203 _aText
_celectronic
300 _aTitle screen
320 _a[References: 25 tit.]
330 _aSequential two-photon ionization is a process that is experimentally accessible due to the use of new free-electron laser sources for excitation. For the prototypical rare Ar gas atoms, a photoelectron spectrum (PES) corresponding to the second step of the sequential two-photon double ionization (2PDIII) at a photon excitation energy of 65.3 eV was studied theoretically with a focus on the consequences of electron correlations in the considered process. The calculation predicts many intense lines at low photoelectron energies, which cannot be explained on the basis of a one-electron approximation. The processes that lead to the appearance of these lines include many-electron correlations, either in the first or second step of photoionization. A significant fraction of the intensity of the low-energy part of PES is associated with the Auger decay of the excited states formed at the second step of 2PDI. The shape of the low-energy part of the 2PDIII PES is expected to be dependent on both the energy of photon excitations and the flux of the exciting beam.
461 _tAtoms
463 _tVol. 10, iss. 4
_v[139, 12 p.]
_d2022
610 1 _aэлектронный ресурс
610 1 _aтруды учёных ТПУ
610 1 _asequential photoionization
610 1 _adouble ionization
610 1 _aphotoelectron spectra
610 1 _aargon
610 1 _amany-electron correlations
610 1 _afree-electron laser
610 1 _aфотоионизация
610 1 _aфотоэлектронные спектры
610 1 _aаргон
701 1 _aLagutin
_bB. M.
_gBoris Mikhaylovich
701 1 _aPetrov
_bI. D.
_gIvan Dmitrievich
701 1 _aSukhorukov
_bV. L.
_gViktor Lvovich
701 1 _aKilin
_bV. A.
_cmathematician
_cProfessor of Tomsk Polytechnic University, doctor of physical and mathematical Sciences
_f1949-
_gViktor Andreevich
_2stltpush
_3(RuTPU)RU\TPU\pers\35524
701 1 _aNovikovsky
_bN. M.
_gNikolay Mikhaylovich
701 1 _aDemekhin
_bF. V.
_gFilipp Vladimirovich
701 1 _aEhresmann
_bA.
_gArno
712 0 2 _aНациональный исследовательский Томский политехнический университет
_bШкола базовой инженерной подготовки
_bОтделение математики и информатики
_h8031
_2stltpush
_3(RuTPU)RU\TPU\col\23555
801 2 _aRU
_b63413507
_c20230410
_gRCR
856 4 _uhttps://doi.org/10.3390/atoms10040139
942 _cCF